Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 133, Issue 20, Pages 7684-7687Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja201813n
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Funding
- WPI Initiative, MEXT, Japan
- JSPS
- Department of Energy, Office of Basic Energy Science
- [21350100]
- Grants-in-Aid for Scientific Research [10J03334, 21350100, 23550207, 22016006] Funding Source: KAKEN
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A bottom-up strategy has been developed to construct a multiple electron transfer system composed of organic/inorganic ternary composites (porphyrin, zinc oxide nanoparticles, reduced graphene oxide) on a semiconducting electrode without impairing the respective donor-acceptor components. The hierarchical electron transfer cascade system exhibited remarkably high photo-current generation with an incident-photon-to-current efficiency of up to ca. 70%.
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