Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 133, Issue 40, Pages 15822-15825Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja205126t
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- National Science Council of Taiwan [NSC 98-2112-M-007-028-MY3, NSC 98-2119-M-002-007-MY3]
- Low Carbon Energy Research Center, National Tsing-Hua University
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A novel donor-acceptor-acceptor (D-A-A) donor molecule, DTDCTB, in which an electron-donating ditolylaminothienyl moiety and an electron-withdrawing dicyanovinylene moiety are bridged by another electron-accepting 2,1,3-benzothiadiazole block, has been synthesized and characterized. A vacuum-deposited organic solar cell employing DTDCTB combined with the electron acceptor C-70 achieved a record-high power conversion efficiency (PCE) of 5.81%. The respectable PCE is attributed to the solar spectral response extending to the near-IR region and the ultracompact absorption dipole stacking of the DTDCTB thin film.
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