Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 1, Pages 67-70Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja208469n
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Funding
- National Basic Research Program of China (973 Program) [2012CB821706]
- National Natural Science Foundation for Distinguished Young Scholars of China [20825102]
- National Natural Science Foundation of China [21171114, 21101103]
- Shantou University
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The gyroid is ubiquitous for underlying the construction of natural substance and artificial zeolites, but it has been, surprisingly, overlooked by chemists who work in the field of metal-organic frameworks (MOFs). In this work, a series of gyroidal MOFs with gie topology, constructed from 1,2-bis((5H-imidazol-4-yl)methylene)hydrazine and octahedral metal ions, such as Zn-II, Mn-II, Cu-II, and Ni-II, have been synthesized. The Zn-II analogue, named as STU-1, shows exceptional thermal and chemical stabilities, and exhibits permanent porosity and CO2 capture ability.
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