Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 133, Issue 39, Pages 15350-15353Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja207386q
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Funding
- NIH (NIGMS) [R01-GM079554, 4R01-GM079554-S1]
- Welch Foundation [I-1596]
- UT Southwestern
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We describe herein an asymmetric synthesis of ageliferin. A Mn(III)-mediated oxidative radical cyclization reaction was used as the key step to construct the core skeleton of this pyrrole-imidazole dimer. This approach resembles the biogenic [4 + 2] dimerization in an intramolecular fashion.
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