Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 2, Pages 800-803Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja209352s
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Funding
- UCB
- BBSRC
- BBSRC [BB/E004350/1] Funding Source: UKRI
- EPSRC [EP/E000614/1, EP/G026688/1, EP/I500200/1] Funding Source: UKRI
- Biotechnology and Biological Sciences Research Council [EGA17763, BB/C510824/1, BB/E004350/1] Funding Source: researchfish
- Engineering and Physical Sciences Research Council [EP/D023343/1, EP/E000614/1, EP/D023335/1, EP/G026688/1, EP/I500200/1, EP/D023327/1, GR/T26542/01] Funding Source: researchfish
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Benign C-C bond formation at various sites in cell-surface channels has been achieved through Suzuki-Miyaura coupling of genetically positioned unnatural amino acids containing aryl halide side chains. This enabled site-selective cell surface manipulation of Escherichia coli; the phosphine-free catalyst caused no cell death at required Pd loadings, suggesting future in vivo application of catalytic metal-mediated bond formation in more complex organisms.
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