Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 133, Issue 21, Pages 8142-8145Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja202791n
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Funding
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059, DE-SC0000989]
- NSF [DMR-0520513]
- JSR Corp. Japan
- European Community [234808]
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We report the synthesis, characterization, and first implementation of a naphtho[2,3-b:6,7-b']dithiophene (NDT)-based donor molecule in highly efficient organic photovoltaics (OPVs). When NDT(TDPP)(2) (TDPP = thiophene-capped diketopyrrolopyrrole) is combined with the electron acceptor PC61BM, a power conversion efficiency (PCE) of 4.06 +/- 0.06% is achieved-a record for a PC61BM-based small-molecule OPV. The substantial PCE is attributed to the broad, high oscillator strength visible absorption, the ordered molecular packing, and an exceptional hole mobility of NDT(TDPP)(2).
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