Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 133, Issue 48, Pages 19362-19365Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja210078d
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Funding
- European Community [FP7/2007-2013, ENHANCE-238409]
- PRIN-COFIN
- Padova University PRAT
- Regione Lombardia-INSTM PICASSO
- ALADIN Industria
- Regione Friuli Venezia (IDROBIM)
- Fondo Trieste
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p-Type Co3O4 nanostructured films are synthesized by a plasma-assisted process and tested in the photocatalytic production of H-2 from water/ethanol solutions under both near-UV and solar irradiation. It is demonstrated that the introduction of fluorine into p-type Co3O4 results in a remarkable performance improvement with respect to the corresponding undoped oxide, highlighting F-doped Co3O4 films as highly promising systems for hydrogen generation. Notably, the obtained yields were among the best ever reported for similar semiconductor-based photocatalytic processes.
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