Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 132, Issue 22, Pages 7559-7567Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja101578m
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Funding
- Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [SISGR-DE-SC0002219]
- National Science Foundation [CHE 0808927]
- Robert A. Welch Foundation [F-0021, H-F-0037]
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This paper offers a perspective on inner-sphere heterogeneous electron-transfer reactions and electrocatalysis as it is applied to electrochemical energy conversion systems. Fundamental concepts and an overview of past approaches to studies of these types of reactions are discussed. A method for the discovery of new electrocatalysts (for example, ones for the oxygen reduction reaction) and photocatalysts (for solar energy conversion to fuels) based on scanning electrochemical microscopy is briefly described, as well as new surface interrogation techniques for quantifying intermediates.
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