Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 132, Issue 12, Pages 4054-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja9109677
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Funding
- AFOSR MURI [FA 9550-06-01-0326]
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Enlarging the molecular size of zinc phthalocyanine (Pc) dyes three dimensionally with 2,6-diphenylphenoxy substituents significantly reduced the aggregation of the dyes on a TiO(2) surface. As a result, the incident photon-to-current conversion efficiency was improved not only in the Q band but over the whole absorption range, achieving 4.6% energy conversion efficiency under one-sun conditions. Electron Lifetime measurements indicated that these Pc dyes do not enhance charge recombination, encouraging further development of Pc.
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