Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 132, Issue 10, Pages 3258-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja100041e
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Funding
- NSF [CHE-0969157]
- NIGMS [R01 GM084254]
- UCSB
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [0969157] Funding Source: National Science Foundation
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An expedient and reliable method for accessing reactive alpha-oxo gold carbenes via gold-catalyzed intermolecular oxidation of terminal alkynes has been developed. Significantly, this method offers a safe and economical alternative to the strategies based on diazo substrates. Its synthetic potential is demonstrated by expedient preparation of dihydrofuran-3-ones containing a broad range of functional groups.
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