Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 132, Issue 37, Pages 12865-12867Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja1066509
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Funding
- MEXT, Japan [19105002]
- JSPS
- Grants-in-Aid for Scientific Research [19105002, 22750090] Funding Source: KAKEN
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Rhodium-catalyzed asymmetric 1,6-addition of arylboronic acids to beta-alkynyl acrylamides substituted with a silyl group on the alkyne terminus took place to give high yields of axially chiral allenylsilanes with 94-99% enantioselectivity, which was realized by use of a rhodium/chiral diene complex.
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