Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 132, Issue 6, Pages 1822-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja909807f
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Funding
- National NSF of China [20972102, 20732003, 20772085]
- PCSIRT [IRT0846]
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An efficient methodology for the synthesis Or unsymmetrical biheteroaryl molecules has been developed via Pd(II)-catalyzed oxidative C-H/C-H cross-coupling, of heteroarenes. An inversion in reactivity and selectivity has been achieved successfully to perform the desired heterocoupling. This process allows the heterocoupling of not only electron-rich N-containing, heteroarenes (e.g., xanthines, azoles, and indolizines) but also electron-poor pyridine N-oxides with various thiophenes or furans.
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