Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 132, Issue 38, Pages 13160-13161Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja106052e
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A new s-tetrazine-based low-bandgap semiconducting polymer, PCPDTTTz, was designed and synthesized. This is the first solution-processable conjugated polymer with tetrazine in the main chain. This polymer shows good thermal stability and broad absorption covering 450-700 nm. The HOMO and LUMO energy levels were estimated to be -5.34 and -3.48 eV, with an electrochemical bandgap of 1.86 eV. Simple polymer solar cells based on PCPDTTTz and PC71BM exhibit a calibrated power conversion efficiency of 5.4%.
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