Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 132, Issue 32, Pages 10955-10957Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja104505t
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Funding
- National Natural Science Foundation of China
- National Basic Research Program of China (973 Program) [2006CB806106, 2010CB833300]
- Ministry of Health [2009ZX09501-017]
- Ministry of Education of China [B06005]
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The nickel-catalyzed reductive coupling of alkynes and imines with Et2Zn as a reductant by using electron-rich phosphine ligands has been developed, affording various allylic amines with high yields and excellent chemoselectivities. Chiral induction was also achieved in this reductive coupling reaction when a nickel catalyst containing a chiral spiro phosphine ligand was used.
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