Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 132, Issue 21, Pages 7306-7311Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja909674e
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Funding
- European Union [MRTN-CT-2006-035810]
- Swiss National Science Foundation
- NCCR 'Nanoscale Science'
- Wolfermann-Nageli Stiftung
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The in vacuo self-assembly of a two-component porphyrin system on a metal surface is studied by means of scanning tunneling microscopy in the sub-monolayer regime. The observed self-assemblies are systematically analyzed by their dependence on the total coverage and on the ratio of the two components resulting in a two-dimensional phase diagram. In a small region within the parameter space, a mixed surface layer is observed. The results are discussed consistently on the basis of molecule surface and molecule molecule interactions as well as thermodynamic aspects, leading to a qualitative comprehension of the phase behavior of the two-dimensional bimolecular system.
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