Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 131, Issue 11, Pages 3840-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja900020a
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Funding
- NSF [CHE-0608664]
- NIH [5R01-GM081546-01]
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A convergent synthesis of the marine natural product (+)-peloruside has been reported. This target has been assembled through the successive application of two methyl, ketone boron aldol addition reactions to the latent C(7)-C(11)-dialdehyde synthon. This approach afforded a 22-step synthesis of this natural product. The influence of resident stereocenters on aldol reaction diastereoselection has been examined in detail.
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