Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 131, Issue 35, Pages 12552-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja905908z
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Funding
- MEXT, Japan [19028015, 20675002, 21.906]
- Grants-in-Aid for Scientific Research [20675002, 19028015] Funding Source: KAKEN
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We have established that a cationic rhodium(I)/(R,R)-QuinoxP(star) complex catalyzes the highly enantioselective direct intermolecular hydroacylation of a-substituted acrylamides with unfunctionalized aliphatic aldehydes to yield the corresponding gamma-ketoamides in high yields with excellent ee values.
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