Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 131, Issue 45, Pages 16366-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja908081s
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Funding
- National Natural Science Foundation of China [20503027, 20773113, 20803072]
- Ministry of Science and Technology of China
- Solar Energy Project of the Chinese Academy of Sciences
- MPG-CAS Partner Group Program
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By rational design of the FeO(111)/Pt(111) inverse model catalyst and the control experiments, we report for the first time direct experimental evidence for the interfacial COads + OHads reaction to produce CO2 at the Pt-oxide interface at low temperatures, providing deep insights into the reaction mechanism and active site of the important tow-temperature water-gas shift and preferential CO oxidation reactions catalyzed by Pt/oxide nanocatalysts at the molecular level.
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