Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 131, Issue 12, Pages 4204-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja900203f
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- U.S. Department of Energy [DE-FG02-03ER15457]
- Northwestern NSEC
- AFOSR
- NSF
- DTRA/ARO
- U.S. Department of Energy (DOE) [DE-FG02-03ER15457] Funding Source: U.S. Department of Energy (DOE)
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Through the use of the tetratopic ligand 1,2,4,5-tetrakis(4-carboxyphenyl)benzene as a key building block, a permanently microporous metal-organic framework with Lewis acidic (porphyrin)Zn struts, ZnPO-MOF, can be made in high yields. ZnPO-MOF can efficiently catalyze acyl-transfer reactions primarily by preconcentrating the substrates within its pores, in stark contrast to analogous supramolecular systems.
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