Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 131, Issue 26, Pages 9186-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja901109t
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Funding
- U.S. Department of Energy [DE-FC36-07GO17033]
- U.S. Defense Logistics Agency [N00164-07-P-1300]
- U.S. National Science Foundation [CHE-0449634]
- [CHE-0535644]
- [DEAC02-06CH 11357]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [0822838] Funding Source: National Science Foundation
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Reactions between two novel hexatopic carboxylate ligands and copper salts give rise to two isostructural metal-organic frameworks (MOFs) with a (3,24)-connected network topology containing both micro- and mesocavities with sizes of up to 3 nm. Both frameworks retain their porosity after guest-molecule removal, leading to high surface areas. Constructing MOFs containing mesocavities with microwindows may serve as a general approach toward stable MOFs with high surface areas.
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