Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 131, Issue 22, Pages 7510-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja901244e
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Funding
- National Science Foundation [0524533]
- STC program [DMR-0120967]
- U.S. Army Research Laboratory [W911NF0420012, 50372-CHMUR]
- U.S. Army Research Office [50372-CHMUR]
- DARPA [MORPH N00014-06-1-0897]
- Directorate For Engineering
- Div Of Electrical, Commun & Cyber Sys [0524533] Funding Source: National Science Foundation
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A chromophore in which zinc porphyrin donors are linked through their meso positions by ethynyl bridges to a bis(indolinylidenemethyl) squaraine core has been synthesized using Sonogashira coupling. The chromophore exhibits a two-photon absorption spectrum characterized by a peak cross section of 11000 GM and, more unusually, also exhibits a large cross section of >780 GM over a photon-wavelength window 750 nm in width.
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