Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 130, Issue 38, Pages 12632-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja805493y
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- NSERC of Canada
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Phosphinoboranes that combine bulky electron-rich phosphides and electron deficient B(C(6)F(5))(2) fragments produce monomeric phosphinoboranes that undergo facile addition of H(2) to give the phosphine-borane adducts (R(2)PH)(HBR'(2)). This finding in combination with DFT calculations shed light on the uptake of H(2) across a group 13-group 15 bond, a critical requirement for the development of recyclable H(2) storage materials.
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