Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 130, Issue 2, Pages 404-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja077457u
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Funding
- EPSRC [EP/D074487/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/D074487/1] Funding Source: researchfish
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We have developed a catalytic enantioselective strategy for chemical synthesis wherein flat aromatic molecules are directly converted to complex nonremmic molecular arch lectures. The process Involves oxidative dearomatization of substituted phenols followed by a desymmebrizing secondry amine-catalyzed asymmetric intermolecular Michael addition and reveals a declin structure formed with exquisite control of three now streogenic centers and an array of exploitable orthogonal functionality directly from a flat molecule that is devoid or architectural complexity.
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