Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 130, Issue 37, Pages 12242-+Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja8046156
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- EPSRC
- Royal Commission for the Exhibition of 1851
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New CO2-philic hydrocarbon molecules were synthesized by reversible addition fragmentation chain-transfer polymerization. These poly(vinyl alkylates) show the highest solubility in supercritical CO2 Of any hydrocarbon reported to date. By utilizing the anchoring ability of the thiocarbonylthio end group, the dispersion polymerization of N-vinyl pyrrolidone was successfully achieved in scCO(2) leading to high yields of well-defined spherical polymer particles.
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