Journal
APPLIED PHYSICS LETTERS
Volume 106, Issue 8, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.4907777
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Funding
- Deutsche Forschungsgemeinschaft [TRR 61]
- Alexander von Humboldt Foundation
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We demonstrate that the Van der Waals interactions in plane are important to control molecular self-assembly structure as well their phase transition. Using precise chemical modification to mediate such in-plane cohesive interactions, we observed the spontaneous formations of 2D order or disorder molecular self-assembly structures, as well their order-disorder phase transitions by annealing. Interestingly, we identified that the side alkyl chains stand up at surfaces and form the 'locked' pairs/windmill structures. Moreover, we realized the covalent coupling based on ethynyl functionality before molecular desorption from metal surfaces, by enhancing the in-plane interactions. (C) 2015 AIP Publishing LLC.
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