Journal
JOURNAL OF SOLID STATE ELECTROCHEMISTRY
Volume 14, Issue 9, Pages 1541-1546Publisher
SPRINGER
DOI: 10.1007/s10008-009-0982-3
Keywords
Dye-sensitized solar cell; Nanocrystallined TiO2; Metal-free organic dye; Counter electrode; Double-walled carbon nanotube (DWCNT)
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Funding
- National Natural Science Foundation of China [10774046]
- Shanghai Municipal Science & Technology Committee [09JC1404600, 0852nm06100, 08230705400]
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Double-walled carbon nanotubes (DWCNTs) have been studied for counter-electrode application in dye-sensitized solar cells (DSCs). Mesoporous TiO2 films are prepared from the commercial TiO2 nanopowders by screen-printing technique on optically transparent-conducting glasses. A metal-free organic dye (indoline dye D102) is used as a sensitizer. DWCNTs are applied to substitute for platinum as counter-electrode materials. Morphological and electrochemical properties of the formed counter electrodes are investigated by scanning electronic microscopy and electrochemical impedance spectroscopy, respectively. The electronic and ionic processes in platinum and DWCNT-based DSCs are analyzed and discussed. The catalytic activity and DSC performance of DWCNTs and Pt are compared. A conversion efficiency of 6.07% has been obtained for DWCNT counter-electrode DSCs. This efficiency is comparable to that of platinum counter-electrode-based devices.
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