Journal
JOURNAL OF SOLID STATE ELECTROCHEMISTRY
Volume 13, Issue 7, Pages 1101-1109Publisher
SPRINGER
DOI: 10.1007/s10008-008-0702-4
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Funding
- Deutsche Forschungsgemeinschaft [Schm 344/34-1, Sa 1770/1-1]
- European Union
- CONICET f
- Swedish Research Council
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Due to progress in the theory of electrocatalysis and in quantum chemistry, it has become possible to investigate the hydrogen reaction and perform quantitative calculations for the reaction rate. First, we demonstrate this with model calculations for the adsorption of hydrogen on Pt(111). In accordance with experimental data, we find hydrogen adsorption at a potential above the equilibrium potential and with an almost vanishing energy of activation. As a second example, we explain trends in the catalytic activity of palladium overlayers and clusters on Au(111) electrodes.
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