Journal
APPLIED PHYSICS EXPRESS
Volume 9, Issue 1, Pages -Publisher
IOP PUBLISHING LTD
DOI: 10.7567/APEX.9.011801
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Funding
- Ministry of Education Culture, Sports, Science and Technology, Japan (MEXT) program Elements Strategy Initiative to Form Core Research Center
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Rechargeable performance is realized in Mg batteries using a TiS3 cathode without the nanometer-scale downsizing of electrode particles. The specific capacity is about 80mAh/g for the first 50 cycles at room temperature. This observed specific capacity is comparable to that of the prototype cathode for Mg batteries. First-principles calculation indicates that TiS3 is a semiconductor with d-p orbital hybridized electronic structures around the Fermi level. The reversible electrode performance is likely assisted by the delocalized electronic distribution over metal-ligand units through d-p orbital hybridization. (C) 2016 The Japan Society of Applied Physics
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