Journal
JOURNAL OF POWER SOURCES
Volume 264, Issue -, Pages 8-14Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2014.04.090
Keywords
Lithium-sulfur; Binder; Poly(vinylpyrrolidone); Poly(ethylene oxide)
Funding
- Era Net Transport project MaLiSu and Vinnova in Sweden
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Binders based on mixtures of poly(ethylene oxide) (PEO) and poly(vinylpyrrolidone) (PVP) are here shown to significantly improve the reversible capacity and capacity retention of lithium- sulfur batteries compared to conventional binders. This mixed binder formulation combines the local improvement to the solvent system offered by PEO and the lithium (poly)sulfide-stabilising effect of PVP. Cells with cathodes made of simple mixtures of sulfur powder and carbon black with a binder of 4:1 PEO:PVP exhibited a reversible capacity of over 1000 mAh g(-1) at C/5 after 50 cycles and 800 mAh g(-1) at 1C after 200 cycles. Furthermore, these materials are water soluble, environmentally friendly and widely available, making them particularly interesting for large-scale production and applications in, for example, electric vehicles. (C) 2014 Elsevier B.V. All rights reserved.
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