Journal
JOURNAL OF POWER SOURCES
Volume 235, Issue -, Pages 220-225Publisher
ELSEVIER
DOI: 10.1016/j.jpowsour.2013.01.084
Keywords
Lithium sulfur battery; Lithium sulfide; Li2S; Carbon coating; PAN
Funding
- VW
- Rockwood Lithium
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In this paper, we investigated the properties of carbon coated lithium sulfide particles prepared following either a dry coating process or a wet coating process, using, respectively, sucrose or polyacrylonitrile (PAN) as carbon source. X-ray diffraction analysis revealed that the crystalline structure of the pristine Li2S was basically preserved upon both coating processes. The dry coating process (Li2S-C-sucrose) resulted in Li2S particles covered only partially by smaller carbon particles, whereas the wet coating method (Li2S-C-PAN) gave Li2S particles, homogenously decorated with thin carbon flakes. As a result, the cycling performance of Li2S-C based electrodes was significantly improved, particularly for Li2S-C-PAN, for which a coulombic efficiency of more than 99.5% was obtained. (C) 2013 Elsevier B.V. All rights reserved.
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