Journal
JOURNAL OF POWER SOURCES
Volume 206, Issue -, Pages 253-258Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2011.12.064
Keywords
Germanium nanowires; Porous carbon; Composite; Solution-liquid-solid; Lithium ion batteries
Funding
- MOE (Singapore) [RG 31/08]
- Singapore Ministry of Education [MOE2010-T2-1-017]
- A*STAR SERC [1021700144]
- [NRF2009EWT-CERP001-026]
- [MPA 23/04.15.03 RDP 009/10/102]
- [MPA 23/04.15.03 RDP 020/10/113]
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Lithium-ion batteries have been actively researched in recent years due to it being one of the most promising energy storage systems. Herein, we report a novel approach where germanium nanowires (Ge NW) are grown in gold-seeded porous carbon via the solution-liquid-solid mechanism, and the corresponding improvement observed in terms of the specific capacity of this porous carbon-germanium nanowires (PC-Ge NW) composite anode. At a current density of 160 mAg(-1) and voltage window of 0.001-1.5 V. a specific capacity of 789 mAhg(-1) during the 50th cycle for PC-Ge NW is achieved as compared to 624 mAhg(-1) during the 50th cycle for pure Ge NW. Even though the content of the Ge is only 53.5 weight percent in the PC-Ge NW composite, it yields a better stability and higher specific capacity, indicating a synergistic effect between porous carbon and Ge nanowires. There is also potential cost savings since the use of a lower amount of Ge can bring about good cycling properties. (C) 2012 Elsevier B.V. All rights reserved.
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