Journal
JOURNAL OF POWER SOURCES
Volume 189, Issue 1, Pages 602-606Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2008.09.088
Keywords
1,3-Propane sultone; Additive; Graphite; Li deposition; Li intercalation
Funding
- National Research Foundation of Korea [과C6B1911] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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1,3-Propane sultone (PS) additive for graphite electrodes was studied for propylene carbonate (PC) and ethylene carbonate (EC)-based electrolytes in lithium batteries. Decomposition of solvents with graphite electrodes could be remarkably suppressed by addition of the PS additive in the PC-based electrolyte, leading to improvement of electrochemical performances of the cells. The 1,3-propane sultone additive showed very interesting properties for the graphite electrode. It is predicted to give a solid electrolyte interphase (SEI) on the surface of the graphite prior to solvent decomposition and bring about effects that not only suppress lithium deposition on the graphite electrode surface, but also accelerate lithium intercalation, leading to formation of LiC6 onto graphite electrode. (C) 2008 Published by Elsevier B.V.
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