Journal
JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY
Volume 48, Issue 4, Pages 743-750Publisher
WILEY
DOI: 10.1002/pola.23824
Keywords
click chemistry; crosslinking; synthesis; thin films; thiol-ene
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Funding
- National Science Foundation, Chemistry Program [CHE-0514031]
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As a tribute to Professor Charlie Hoyle, we take the opportunity to review the impact of thiol-ene chemistry on polymer and materials science over the past 5 years. During this time, a renaissance in thiol-ene chemistry has occurred with recent progress demonstrating its unique advantages when compared with traditional coupling and functionalization strategies. Additionally, the robust nature of thiol-ene chemistry allows for the preparation of well-defined materials with few structural limitations and synthetic requirements. To illustrate these features, the utility of thiol-ene reactions for network formation, polymer functionalization, dendrimer synthesis, and the decoration of three-dimensional objects is discussed. Also, the development of the closely related thiol-yne chemistry is described. (C) 2010 Wiley Periodicals, Inc. J Polym Sci Part A: Polym Chem 48:743-750, 2010
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