4.5 Article

The Jeff=1/2 insulator Sr3Ir2O7 studied by means of angle-resolved photoemission spectroscopy

Journal

JOURNAL OF PHYSICS-CONDENSED MATTER
Volume 24, Issue 41, Pages -

Publisher

IOP PUBLISHING LTD
DOI: 10.1088/0953-8984/24/41/415602

Keywords

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Funding

  1. Knut and Alice Wallenberg Foundation
  2. Swedish Research Council
  3. Swiss National Science Foundation, its NCCR MaNEP and Sinergia network MPBH
  4. EPSRC
  5. EPSRC [EP/J016713/1, EP/J017124/1] Funding Source: UKRI
  6. Engineering and Physical Sciences Research Council [EP/J017124/1, EP/J016713/1] Funding Source: researchfish

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The low-energy electronic structure of the J(eff) = 1/2 spin-orbit insulator Sr3Ir2O7 has been studied by means of angle-resolved photoemission spectroscopy. A comparison of the results for bilayer Sr3Ir2O7 with available literature data for the related single-layer compound Sr2IrO4 reveals qualitative similarities and similar J(eff) = 1/2 bandwidths for the two materials, but also pronounced differences in the distribution of the spectral weight. In particular, photoemission from the J(eff) = 1/2 states appears to be suppressed. Yet, it is found that the Sr3Ir2O7 data are in overall better agreement with band-structure calculations than the data for Sr2IrO4.

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