Magnetic excitations of Fe1+ySexTe1-x in magnetic and superconductive phases

We have used inelastic neutron scattering and muon-spin rotation to compare the low energy magnetic excitations in single crystals of superconducting Fe1.01Se0.50Te0.50 and non-superconducting Fe1.10Se0.25Te0.75. We confirm the existence of a spin resonance in the superconducting phase of Fe1.01Se0.50Te0.50, at an energy of 7 meV and a wavevector of (1/2, 1/2, 0). The non-superconducting sample exhibits two incommensurate magnetic excitations at (1/2, 1/2, 0) +/- (0.18, -0.18, 0) which rise steeply in energy, but no resonance is observed at low energies. A strongly dispersive low energy magnetic excitation is also observed in Fe1.10Se0.25Te0.75 close to the commensurate antiferromagnetic ordering wavevector (1/2 - delta, 0, 1/2), where delta approximate to 0.03. The magnetic correlations in both samples are found to be quasi-two-dimensional in character and persist well above the magnetic (Fe1.10Se0.25Te0.75) and superconducting (Fe1.01Se0.50Te0.50) transition temperatures.