Journal
PHYSICAL REVIEW LETTERS
Volume 114, Issue 12, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.114.123004
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Funding
- Max Planck Society
- DFG [SFB652/3]
- Cluster of Excellence: Munich Centre for Advanced Photonics (MAP)
- Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U. S. Department of Energy [DE-SC0008146]
- DEFG02- 86ER13491
- National Research Foundation of Korea (NRF) - Ministry of Science, ICT and Future Planning via Global Research Laboratory Program [200900439]
- Max Planck POSTECH/KOREA Research Initiative Program [2011-0031558]
- FWF (Austria) [SFB-041 ViCoM, FB-049 Next Lite, P21141-N16]
- International Max Planck Research School of Advanced Photon Science
- Fonds National de la Recherche
- Fonds National de la Recherche Collective of Belgium [2.4545]
- Einstein Foundation (Berlin)
- Austrian Science Fund (FWF) [P 23359] Funding Source: researchfish
- National Research Foundation of Korea [2011-0031558, 2009-00439] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
- Austrian Science Fund (FWF) [P23359] Funding Source: Austrian Science Fund (FWF)
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Strong laser fields can be used to trigger an ultrafast molecular response that involves electronic excitation and ionization dynamics. Here, we report on the experimental control of the spatial localization of the electronic excitation in the C-60 fullerene exerted by an intense few-cycle (4 fs) pulse at 720 nm. The control is achieved by tailoring the carrier-envelope phase and the polarization of the laser pulse. We find that the maxima and minima of the photoemission-asymmetry parameter along the laser-polarization axis are synchronized with the localization of the coherent electronic wave packet at around the time of ionization.
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