Journal
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume 4, Issue 10, Pages 1597-1602Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jz400659b
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Funding
- Spanish Ministerio de Economia y Competitividad (MINECO) [CTQ2011-27317]
- Comunidad de Madrid [S2009/MAT-1726, S2009/PPQ-1533]
- Ramon y Cajal grant of the MINECO
- EC Amarout grant [2295]
- Basic Science Research Program (CRI) [RIAMI-AM0209(0417-20090011)]
- WCU (World Class University) project through National Research Foundation of Korea [R31-2008-000-10075-0]
- Ministry of Education, Science and Technology
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J-aggregation has been shown to be beneficial for light amplification in single crystals of pi-conjugated organic molecules. In the case of H-aggregation, the criteria for such processes are still under debate. It has also been shown that H-aggregate arrangements with considerable pi-pi overlap are detrimental for light amplification. We show here that a proper alignment of the molecules in the crystal lattice, which minimizes pi-pi overlap between adjacent molecules, gives rise to (random) stimulated emission from cofacial arrangements similar to that of the herringbone aggregates.
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