Journal
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume 4, Issue 22, Pages 3853-3856Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jz402100g
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Funding
- Austrian Science Funds FWF [M1404, I1115-N19]
- European Union through the EFRE INTERREG IV (ETC-AT-CZ) program [M00146]
- US NSF [CHE 0957586]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [0957586] Funding Source: National Science Foundation
- Austrian Science Fund (FWF) [M1404] Funding Source: Austrian Science Fund (FWF)
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We introduce two-dimensional NMR spectroscopy detected by recording and processing the noise originating from nuclei that have not been subjected to any radio frequency excitation. The method relies on cross-correlation of two noise blocks that bracket the evolution and mixing periods. While the sensitivity of the experiment is low in conventional NMR setups, spin-noise-detected NMR spectroscopy has great potential for use with extremely small numbers of spins, thereby opening a way to nanoscale multidimensional NMR spectroscopy.
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