Journal
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume 3, Issue 17, Pages 2442-2446Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jz301013u
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Funding
- Swedish Energy Agency (STEM)
- Swedish Research Council
- European Research Council [226136-VISCHEM]
- Knut&Alice Wallenberg foundation
- Academy of Sciences of the Czech Republic [M100101218]
- European Community
- Serbian Ministry of Science [ON171017]
- FP7 project PRACE-IIP
- FP7 project PRACE-2IP
- FP7 project HP-SEE
- FP7 project EGI-InSPIRE
- EC FP7 ONE-P project
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Time-resolved terahertz spectroscopy was employed for the investigation of charge-transport dynamics in benzothiadiazolo-dithiophene polyfluorene ([2,7-(9,9-dioctylfluorene)-alt-S,S-(4',7'-di-2-thieny1-2',1',3'-benzothiadiazole)]) (APFO-3) polymers with various chain lengths and in its monomer form, all blended with an electron acceptor ([6,6]-phenyl-C61-butyric acid methyl ester, PCBM). Upon photo-excitation, charged polaron pairs are created, negative charges are transferred to fullerenes, while positive polarons remain on polymers/monomers. Vastly different hole mobility in polymer and monomer blends allows us to distinguish the hole and electron contributions to the carrier mobility.
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