Journal
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume 3, Issue 10, Pages 1248-1252Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jz3003316
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Funding
- Ministry of Education, Culture, Sports, Science, and Technology of Japan [470, 19049001, 23225006]
- Low-Carbon Research Network of Japan
- Grants-in-Aid for Scientific Research [23225006, 23686026, 24655162, 24107003, 23655167] Funding Source: KAKEN
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We report the stoichiometric evolution of oxygen via water oxidation by irradiating a plasmon-enhanced photocurrent generation system with near-infrared light (lambda: 1000 am), in which gold nanostructures were arrayed on the surface of TiO2 electrode. It is considered that multiple electron holes generated by plasmon-induced charge excitation led to the effective recovery of water oxidation after the electron transfer from gold to TiO2. The proposed system containing a gold nanostructured TiO2 electrode may be a promising artificial photosynthetic system using near-infrared light.
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