Journal
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume 3, Issue 17, Pages 2326-2331Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jz300981w
Keywords
-
Categories
Funding
- Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy
- National Science Foundation [CHE-1058791]
- National Institutes of Health [GM-59230]
- EMSL at PNNL
- Direct For Mathematical & Physical Scien [1058791] Funding Source: National Science Foundation
- Division Of Chemistry [1058791] Funding Source: National Science Foundation
Ask authors/readers for more resources
We show that broadband X-ray pulses can create wavepackets of valence electrons and holes localized in the vicinity of a selected atom (nitrogen, oxygen, or sulfur in cysteine) by stimulated resonant Raman scattering. The subsequent dynamics reveals highly correlated motions of entangled electron and hole quasiparticles. This information goes beyond the time-dependent total charge density derived from X-ray diffraction.
Authors
I am an author on this paper
Click your name to claim this paper and add it to your profile.
Reviews
Recommended
No Data Available