Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 118, Issue 8, Pages 4303-4308Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp4093332
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Funding
- Ministry of Education, Culture, Sports, Science, and Technology (MEXT)
- Japan Society for the Promotion of Science (JSPS)
- Grants-in-Aid for Scientific Research [23225005] Funding Source: KAKEN
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Thin films of a thiazyl biradical, naphtho[2,1-d:6,5-d']bis([1,2,3]dithiazole), abbreviated as NT, exhibit nonlinear optical properties with a large third-order nonlinear susceptibility of 2.1 X 10(-11) esu. The electroabsorption and low-temperature-absorption measurements reveal a series of degenerate electronic states, which is probably caused by the biradical character of NT. It is concluded that this degeneracy should enhance the third-order nonlinear optical properties.
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