4.6 Article

Nonlocal Effects in Energy Absorption of Coupled Quantum Dot-Metal Nanoparticle Systems

Journal

JOURNAL OF PHYSICAL CHEMISTRY C
Volume 116, Issue 44, Pages 23663-23670

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/jp3090183

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We theoretically study the optical properties of a hybrid nanostructure consisting of a metal nanoparticle and a semiconductor quantum dot. We derive a closed-form solution for the energy absorption spectra of the hybrid system and investigate the impact of the nonlocal dielectric response of a metal nanoparticle on the energy absorption. The results show significant modification when compared to those obtained with a local dielectric function. More specifically, the magnitude and shape of the energy absorption rate spectra are strongly modified, especially for small interparticle distances and high intensities of an external electric field interacting with the system.

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