Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 114, Issue 8, Pages 3454-3458Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp911629j
Keywords
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Funding
- National Research Laboratory Program [R0A-2008-000-20057-0]
- World Class University (WCU) [R32-2008-000-10051-0]
- pioneer research center program [2009-0093758]
- Korean government [R11-2008-058-03002-0]
- KAIST SEWS [EEWS0903]
- NSF [CMMI-0802247, CMMI-0742065]
- Ministry of Education, Science & Technology (MoST), Republic of Korea [N01090034] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
- National Research Foundation of Korea [2008-0062204, R32-2008-000-10051-0, 2008-0060005, R11-2008-058-03002-0] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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We present a simple model for the growth and termination of carbon nanotube (CNT) arrays. This model was developed by modifying several submodels and provides a comprehensive predictive tool for the CNT growth process as a function of CNT wall number. Wall number, diameter, and areal density-controlled CNT arrays were grown on a reduced graphene film by combining block copolymer lithography and plasma-enhanced chemical vapor deposition (PECVD) method. The number of carbonaceous platelets required for the termination of CNT growth process was measured by high-resolution transmission electron microscopy (HRTEM), and the effective exposed catalyst surface area was measured by high magnification scanning electron microscopy (SEM). A parametric study showed that our simple kinetic model successfully predicted the kinetics of wall number-dependent CNT growth and could be used to optimize the PECVD process for CNT production.
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