Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 113, Issue 8, Pages 3037-3040Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp810319v
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We present a spatiotemporal operando X-ray absorption study of a highly dynamic process, the ignition of the noble metal catalyzed partial oxidation of methane. Evolvement and propagation of the platinum component's structural changes are investigated with a high-speed X-ray camera, which in combination with temperature profiling by IR-thermography and catalytic activity measurements by online mass spectrometry gives insight into the first stages of the ignition of the reaction toward hydrogen and carbon monoxide.
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