Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 113, Issue 39, Pages 16839-16842Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp907377h
Keywords
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Funding
- National Science Foundation [EEC-0118025, CHE-0414554, BES-0507036, DMR-0520513, CHE-0911145]
- National Cancer Institute [1 U54 CAI 19341-01]
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A wide-field localized surface plasmon resonance (LSPR) imaging method using a liquid crystal tunable filter is used to measure the scattering spectra of multiple Ag nanoparticles in parallel. This method provides the ability to characterize moving Ag nanoparticles by measuring the scattering spectra of the particles while Simultaneously tracking their motion. Consequently, single-particle diffusion coefficients can be determined. As an example, several single Ag nanoprisms are tracked, the LSPR scattering spectrum of each moving particle is obtained, and the single-particle diffusion coefficient is determined from its trajectory. Coupling diffusion information with spectral information in real time is a significant advance and addresses many scientific problems, both fundamental and biological, such as cell membrane protein diffusion, functional plasmonic distributions, and nanoparticle growth mechanisms.
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