Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 112, Issue 50, Pages 20095-20098Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp8074145
Keywords
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Funding
- National Natural Science Foundation [20473029, 20573041]
- Program for Changjiang Scholars and Innovative Research Team in University (PCSIRT)
- Program for New Century Excellent Talents in University (NCET)
- Innovative Scholars of Jilin University [2004CX035]
- Fund for the Doctoral Program of Higher Education [20040183048]
- Scientific Research Foundation for the Returned Overseas Chinese Scholars initiated by State Education Ministry
- Program of Introducing Talents of Discipline to Universities [1306009]
- Scientific and Technical Project of Jiamusi University [S2008-045]
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Surface-enhanced Raman scattering from molecules adsorbed on TiO2 nanoparticles has been observed. This is attributed to the dominant contribution of the TiO2-to-molecule charge-transfer mechanism. The charge-transfer process is largely dependent on the intrinsic nature of the adsorbed molecules and the surface properties of the semiconductor. Both the stronger electron attracting ability of groups para- to the mercapto group bonded with TiO2 surface and the plentiful surface states of TiO2 nanoparticles are favorable to TiO2-to-molecule charge-transfer and SERS for molecules adsorbed on TiO2.
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