Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 112, Issue 25, Pages 9124-9127Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp803386g
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The first observation of state-resolved exciton-phonon couplings are reported for the lowest four eigenstates in strongly confined colloidal quantum dots for both optical and acoustic phonons. State-resolved pump/probe experiments show that the excitonic eigenstate has a strong influence upon the Frohlich coupling to optical phonons and a moderate influence on the deformation potential coupling to acoustic phonons. These experiments provide a general approach to measuring exciton-phonon couplings in quantum dots with eigenstate-specificity.
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