Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 112, Issue 46, Pages 17772-17774Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp8078277
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The coadsorption of alkalis with CO and O on Cu(111) and Ni(111) was studied by vibrational measurements. Unexpectedly, we found an enhanced alkali oxidation rate for alkali + CO compared with alkali + O. Such finding was ascribed to the short-range alkali-CO interaction which lowers the barrier for CO dissociation and favors a giant alkali oxidation. Surprisingly, no alkali-O bond was formed for O/alkalis.
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