Journal
PHYSICAL REVIEW E
Volume 92, Issue 2, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevE.92.023017
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Funding
- Collaborative Research Fund of the Hong Kong Special Administrative Region [HKUST9/CRF/11G]
- Postgraduate Scholarship through the Energy Technology Concentration at HKUST
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Molecular dynamics simulations are conducted to study the flow behavior of CsF solutions in nanochannels under external electric fields E. It is found that the channel surface energy greatly affects the flow behavior. In channels of high surface energy, water molecules, on average, move in the same direction as that of the electric field regardless of the strength of E. In low surface energy channels, however, water transports in the opposite direction to the electric field at weak E and the flow direction is changed when E becomes sufficiently large. The direction change of water flow is attributed to the coupled effects of different water-ion interactions, inhomogeneous water viscosity, and ion distribution changes caused by the electric field. The flow direction change observed in this work may be employed for flow control in complex micro- or nanofluidic systems.
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